N1phenethyl-norcymserine, a selective butyrylcholinesterase inhibitor, increases acetylcholine release in rat cerebral cortex: a comparison with donepezil and rivastigmine

Eur J Pharmacol. 2007 Oct 31;572(2-3):142-50. doi: 10.1016/j.ejphar.2007.06.053. Epub 2007 Jul 4.

Abstract

The effects of (-)-N(1)phenethyl-norcymserine (PEC, 5 mk/kg, i.p.) on acetylcholine release and cholinesterase activity in the rat cerebral cortex were compared with those of donepezil (1 mg/kg, i.p.), a selective acetylcholinesterase inhibitor, and rivastigmine (0.6 mg/kg, i.p.), an inhibitor of acetylcholinesterase and butyrylcholinesterase. Acetylcholine extracellular levels were measured by microdialysis coupled with HPLC; acetylcholinesterase and butyrylcholinesterase activity were measured with colorimetric and radiometric methods. It was found that comparable 2-3 fold increases in cortical extracellular acetylcholine level, calculated as areas under the curve, followed the administration of the three drugs at the doses used. At the peak of acetylcholine increase, a 27% acetylcholinesterase inhibition and no butyrylcholinesterase inhibition was found after donepezil (1 mg/kg, i.p) administration. At the same time point, rivastigmine (0.6 mg/kg, i.p.) inhibited acetylcholinesterase by 40% and butyrylcholinesterase by 25%. After PEC (5 mg/kg, i.p.) administration, there was a 39% butyrylcholinesterase inhibition and no effect on acetylcholinesterase. Since in the present study it was also confirmed that in the brain butyrylcholinesterase activity is only about 10% of acetylcholinesterase activity, it is surprising that its partial inhibition is sufficient to increase extracellular acetylcholine levels. The importance of butyrylcholinesterase as a "co-regulator" of synaptic acetylcholine levels should thus be reconsidered.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylcholinesterase / metabolism*
  • Animals
  • Butyrylcholinesterase / metabolism*
  • Cerebral Cortex / drug effects*
  • Cerebral Cortex / metabolism
  • Cholinesterase Inhibitors / metabolism
  • Cholinesterase Inhibitors / pharmacology*
  • Donepezil
  • Dose-Response Relationship, Drug
  • Indans / metabolism
  • Indans / pharmacology*
  • Male
  • Mass Spectrometry
  • Microdialysis
  • Phenylcarbamates / metabolism
  • Phenylcarbamates / pharmacology*
  • Physostigmine / analogs & derivatives*
  • Physostigmine / pharmacology
  • Piperidines / metabolism
  • Piperidines / pharmacology*
  • Rats
  • Rats, Wistar
  • Rivastigmine

Substances

  • Cholinesterase Inhibitors
  • Indans
  • N(1)-phenethylnorcymserine
  • Phenylcarbamates
  • Piperidines
  • Donepezil
  • Physostigmine
  • Acetylcholinesterase
  • Butyrylcholinesterase
  • Rivastigmine