PqsA is required for the biosynthesis of 2,4-dihydroxyquinoline (DHQ), a newly identified metabolite produced by Pseudomonas aeruginosa and Burkholderia thailandensis

Biol Chem. 2007 Aug;388(8):839-45. doi: 10.1515/BC.2007.100.

Abstract

A new metabolite, 2,4-dihydroxyquinoline (DHQ), was identified in cultures of the bacteria Pseudomonas aeruginosa and Burkholderia thailandensis. We found that the biosynthesis of DHQ correlates with the presence of a functional PqsA, which is a product of the pqsABCDE operon responsible for the synthesis of 4-hydroxy-2-alkylquinolines (HAQs) in P. aeruginosa. However, DHQ is not a degradation product or precursor of HAQs. This finding sheds some light on the poorly understood biosynthesis pathway of HAQs, which includes important communication signals regulating the expression of virulence factors.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacterial Proteins / metabolism*
  • Burkholderia / genetics
  • Burkholderia / metabolism*
  • Chromatography, Liquid
  • Genes, Bacterial
  • Mass Spectrometry
  • Oxyquinoline / analysis
  • Oxyquinoline / chemistry
  • Oxyquinoline / metabolism*
  • Pseudomonas aeruginosa / genetics
  • Pseudomonas aeruginosa / metabolism*
  • Quinolines / analysis
  • Quinolines / chemistry
  • Quinolines / metabolism*
  • Stereoisomerism

Substances

  • Bacterial Proteins
  • Quinolines
  • Oxyquinoline
  • 2,4-dihydroxyquinoline