A dual sensor spin trap for use with EPR spectroscopy

Org Lett. 2007 Aug 30;9(18):3499-502. doi: 10.1021/ol071285o. Epub 2007 Aug 1.

Abstract

Redox active metal ions, carbon-centered radicals, and oxygen-centered radicals are important to oxidative stress. A radical detector combining a nitrone spin trap, a phenol, and a cyclopropane radical clocklike unit was prepared and used with EPR spectroscopy to detect and distinguish between hydroxyl radicals, methyl radicals, and iron(III) ions. Iron(III) reacts with the phenol unit inducing opening of the cyclopropane ring and cyclization to generate a stable nitroxyl radical.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cyclopropanes / chemistry*
  • Electron Spin Resonance Spectroscopy / methods*
  • Free Radicals / analysis*
  • Free Radicals / chemistry
  • Molecular Structure
  • Nitrogen Oxides / chemistry*
  • Phenols / chemistry*
  • Spin Trapping

Substances

  • Cyclopropanes
  • Free Radicals
  • Nitrogen Oxides
  • Phenols
  • nitrones
  • cyclopropane