Mild and efficient Lewis acid-promoted detritylation in the synthesis of N-hydroxy amides: a concise synthesis of (-)-Cobactin T

J Org Chem. 2007 Oct 12;72(21):8123-6. doi: 10.1021/jo701411d. Epub 2007 Sep 19.

Abstract

An efficient, high-yielding Lewis acid promoted deprotection of O-trityl hydroxylamine derivatives is described. A range of acid-labile protecting groups, such as N-Boc and O-TBS, were tolerated under these mild conditions. The present method is applicable to the synthesis of a broad range of hydroxylamine derivatives, including N-hydroxy amides (hydroxamic acids), N-hydroxy sulfonamides, and N-hydroxy ureas, which often exhibit significant biological activities. An application of this methodology for a concise synthesis of (-)-Cobactin T (18) is also demonstrated.

MeSH terms

  • Azepines / chemical synthesis*
  • Azepines / chemistry
  • Hydroxamic Acids / chemistry
  • Hydroxylamines / chemical synthesis*
  • Hydroxylamines / chemistry
  • Indicators and Reagents
  • Molecular Structure
  • Trityl Compounds / chemistry*

Substances

  • Azepines
  • Hydroxamic Acids
  • Hydroxylamines
  • Indicators and Reagents
  • Trityl Compounds
  • cobactin T