Huge transverse magnetic polarization in the field-induced phase of the antiferromagnetic molecular wheel CsFe(8)

Phys Rev Lett. 2007 Aug 24;99(8):087201. doi: 10.1103/PhysRevLett.99.087201. Epub 2007 Aug 22.

Abstract

The 1H NMR spectrum and nuclear relaxation rate T(1)(-1) in the antiferromagnetic wheel CsFe8 were measured to characterize the previously observed magnetic field-induced low-temperature phase around the level crossing at 8 T. The data show that the phase is characterized by a huge staggered transverse polarization of the electronic Fe spins, and the opening of a gap, providing microscopic evidence for the interpretation of the phase as a field-induced magnetoelastic instability.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cold Temperature*
  • Magnetic Fields*
  • Magnetic Resonance Spectroscopy