Critical factors to high thermostability of an alpha-amylase from hyperthermophilic archaeon Thermococcus onnurineus NA1

J Microbiol Biotechnol. 2007 Aug;17(8):1242-8.

Abstract

Genomic analysis of a hyperthermophilic archaeon, Thermococcus onnurineus NA1 [1], revealed the presence of an open reading frame consisting of 1,377 bp similar to alpha-amylases from Thermococcales, encoding a 458-residue polypeptide containing a putative 25-residue signal peptide. The mature form of the alpha-amylase was cloned and the recombinant enzyme was characterized. The optimum activity of the enzyme occurred at 80 degrees C and pH 5.5. The enzyme showed a liquefying activity, hydrolyzing maltooligosaccharides, amylopectin, and starch to produce mainly maltose (G2) to maltoheptaose (G7), but not pullulan and cyclodextrin. Surprisingly, the enzyme was not highly thermostable, with half-life (t(1/2)) values of 10 min at 90 degrees C, despite the high similarity to alpha-amylases from Pyrococcus. Factors affecting the thermostability were considered to enhance the thermostability. The presence of Ca2+ seemed to be critical, significantly changing t(1/2) at 90 degrees C to 153 min by the addition of 0.5 mM Ca2+. On the other hand, the thermostability was not enhanced by the addition of Zn2+ or other divalent metals, irrespective of the concentration. The mutagenetic study showed that the recovery of zinc-binding residues (His175 and Cys189) enhanced the thermostability, indicating that the residues involved in metal binding is very critical for the thermostability.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Amino Acid Substitution / genetics
  • Archaeal Proteins / chemistry*
  • Archaeal Proteins / genetics
  • Archaeal Proteins / metabolism
  • Calcium / pharmacology
  • Cations, Divalent / pharmacology
  • Cloning, Molecular
  • Coenzymes / pharmacology
  • DNA, Archaeal / chemistry
  • DNA, Archaeal / genetics
  • Enzyme Stability / genetics*
  • Gene Expression
  • Glucans / metabolism
  • Half-Life
  • Hydrogen-Ion Concentration
  • Molecular Sequence Data
  • Mutagenesis, Site-Directed
  • Oligosaccharides / metabolism
  • Polysaccharides / metabolism
  • Recombinant Proteins / genetics
  • Recombinant Proteins / isolation & purification
  • Recombinant Proteins / metabolism
  • Sequence Alignment
  • Sequence Analysis, DNA
  • Substrate Specificity
  • Temperature
  • Thermococcus / enzymology*
  • Thermococcus / genetics
  • alpha-Amylases / chemistry*
  • alpha-Amylases / genetics
  • alpha-Amylases / metabolism

Substances

  • Archaeal Proteins
  • Cations, Divalent
  • Coenzymes
  • DNA, Archaeal
  • Glucans
  • Oligosaccharides
  • Polysaccharides
  • Recombinant Proteins
  • maltooligosaccharides
  • maltoheptaose
  • alpha-Amylases
  • Calcium

Associated data

  • GENBANK/DQ144136