Theoretical study of ethidium intercalation in triple-stranded DNA and at triplex-duplex junctions

J Biomol Struct Dyn. 1991 Dec;9(3):425-436. doi: 10.1080/07391102.1991.10507926.

Abstract

The contribution of different factors in the interaction of ethidium intercalated into various sequences of a triple helix, or in the region of the junction between the double- and triple-stranded DNA has been studied by energy minimization. It is found that in the total energy of the ethidium- triple helix complexes, a particular electrostatic contribution emerges due to the presence of protonated cytosines in the triple helix. This parameters is determinant in the sequence-specificity of ethidium binding to the triple helix. The preferred intercalation sites of ethidium in the triple helix are proposed. The interaction of ethidium at the triplex-duplex junction, and its effects are also discussed. This study is aimed at searching for new drugs specific for the triple helix, or for the triplex-duplex junctions.

MeSH terms

  • Base Sequence
  • DNA / chemistry*
  • DNA / ultrastructure
  • Deoxyribonucleotides / chemistry
  • Ethidium / chemistry*
  • Hydrogen Bonding
  • Intercalating Agents / chemistry*
  • Molecular Sequence Data
  • Nucleic Acid Conformation
  • Purine Nucleotides / chemistry
  • Pyrimidine Nucleotides / chemistry
  • Sequence Homology, Nucleic Acid
  • Software
  • Thermodynamics

Substances

  • Deoxyribonucleotides
  • Intercalating Agents
  • Purine Nucleotides
  • Pyrimidine Nucleotides
  • DNA
  • Ethidium