Degradation of 4-fluorophenol by Arthrobacter sp. strain IF1

Appl Microbiol Biotechnol. 2008 Mar;78(4):709-17. doi: 10.1007/s00253-008-1343-3. Epub 2008 Jan 29.

Abstract

A Gram-positive bacterial strain capable of aerobic biodegradation of 4-fluorophenol (4-FP) as the sole source of carbon and energy was isolated by selective enrichment from soil samples collected near an industrial site. The organism, designated strain IF1, was identified as a member of the genus Arthrobacter on the basis of 16S ribosomal RNA gene sequence analysis. Arthrobacter strain IF1 was able to mineralize 4-FP up to concentrations of 5 mM in batch culture. Stoichiometric release of fluoride ions was observed, suggesting that there is no formation of halogenated dead-end products during 4-FP metabolism. The degradative pathway of 4-FP was investigated using enzyme assays and identification of intermediates by gas chromatography (GC), GC-mass spectrometry (MS), high-performance liquid chromatography, and liquid chromatography-MS. Cell-free extracts of 4-FP-grown cells contained no activity for catechol 1,2-dioxygenase or catechol 2,3-dioxygenase, which indicates that the pathway does not proceed through a catechol intermediate. Cells grown on 4-FP oxidized 4-FP, hydroquinone, and hydroxyquinol but not 4-fluorocatechol. During 4-FP metabolism, hydroquinone accumulated as a product. Hydroquinone could be converted to hydroxyquinol, which was further transformed into maleylacetic acid and beta-ketoadipic acid. These results indicate that the biodegradation of 4-FP starts with a 4-FP monooxygenase reaction that yields benzoquinone, which is reduced to hydroquinone and further metabolized via the beta-ketoadipic acid pathway.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Arthrobacter / classification
  • Arthrobacter / genetics
  • Arthrobacter / isolation & purification*
  • Arthrobacter / metabolism*
  • Biodegradation, Environmental
  • DNA, Bacterial / genetics
  • DNA, Ribosomal / genetics
  • Gas Chromatography-Mass Spectrometry
  • Hydroquinones / metabolism
  • Molecular Sequence Data
  • Phenols / analysis
  • Phenols / metabolism*
  • Phylogeny
  • RNA, Ribosomal, 16S / genetics
  • Soil Microbiology*

Substances

  • DNA, Bacterial
  • DNA, Ribosomal
  • Hydroquinones
  • Phenols
  • RNA, Ribosomal, 16S
  • 4-fluorophenol
  • hydroquinone

Associated data

  • GENBANK/DQ425093