A conserved cysteine motif essential for ceramide kinase function

Biochimie. 2008 Oct;90(10):1560-5. doi: 10.1016/j.biochi.2008.07.001. Epub 2008 Jul 10.

Abstract

Ceramide kinase (CerK) is a sphingolipid metabolizing enzyme very sensitive to oxidation; however, the determinants are unknown. We show here that the thiol-modifying agent N-ethyl-maleimide abrogates CerK activity in vitro and in a cell based assay, implying that important cysteine residues are accessible in purified as well as endogenous CerK. We replaced every 22 residues in human CerK, by an alanine, and measured activity in the resulting mutant proteins. This led to identification of a cluster of cysteines, C(347)XXXC(351)XXC(354), essential for CerK function. These findings are discussed based on homology modeling of the catalytic domain of CerK.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Motifs
  • Amino Acid Sequence
  • Animals
  • COS Cells
  • Catalytic Domain
  • Chlorocebus aethiops
  • Conserved Sequence*
  • Cysteine / metabolism*
  • Humans
  • Molecular Sequence Data
  • Oxidation-Reduction
  • Phosphotransferases (Alcohol Group Acceptor) / chemistry*
  • Phosphotransferases (Alcohol Group Acceptor) / metabolism*
  • Sulfhydryl Compounds

Substances

  • Sulfhydryl Compounds
  • Phosphotransferases (Alcohol Group Acceptor)
  • ceramide kinase
  • Cysteine