Anti-inflammatory activity of the extracts and fractions from Erigeron multiradiatus through bioassay-guided procedures

J Ethnopharmacol. 2008 Sep 26;119(2):232-7. doi: 10.1016/j.jep.2008.06.035. Epub 2008 Jul 10.

Abstract

Ethnopharmacological relevance: Erigeron multiradiatus (Lindl.) Benth., an herb that grows in the alpine and subalpine meadow of Qinghai-Tibet plateau, has been widely used as a folk remedy by the native people for treatment of various inflammatory ailments.

Aim of the study: In order to isolate and identify the active components of Erigeron multiradiatus for anti-inflammatory activity, a preliminary phytochemical study and a bioassay-guided fractionation and purification process was performed.

Material and methods: The dry whole plant Erigeron multiradiatus was extracted with 50% ethanol and then separated into CHCl(3), n-BuOH, and aqueous fractions. The anti-inflammatory activities of each fraction were investigated using two in vivo inflammation models.

Results: These results exhibited varying degrees of anti-inflammatory activities and the n-BuOH fraction showed the strongest anti-inflammatory activities. The n-BuOH fraction was then subjected to separation and purification using macroporous resins column chromatography and Sephadex LH-20 leading to two flavonoids glucuronides identified as scutellarein-7-O-beta-glucuronide and apigenin-7-O-beta-glucuronide. Furthermore, LC-MS/MS identification and quantification of isolated compounds were also performed.

Conclusion: Scutellarein-7-O-beta-glucuronide and apigenin-7-O-beta-glucuronide were considered as major components and principally responsible for the anti-inflammatory activity of Erigeron multiradiatus. Thus the results of our study provide a scientific basis for the utilization of Erigeron multiradiatus in traditional Tibetan medicine.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anti-Inflammatory Agents / isolation & purification
  • Anti-Inflammatory Agents / pharmacology*
  • Apigenin / isolation & purification
  • Apigenin / pharmacology
  • Biological Assay / methods
  • Disease Models, Animal
  • Edema / drug therapy
  • Erigeron / chemistry*
  • Female
  • Flavonoids / isolation & purification
  • Flavonoids / pharmacology
  • Glucuronates / isolation & purification
  • Glucuronates / pharmacology
  • Inflammation / drug therapy*
  • Male
  • Medicine, Tibetan Traditional
  • Mice
  • Plant Extracts / pharmacology*
  • Rats
  • Rats, Sprague-Dawley
  • Tibet

Substances

  • Anti-Inflammatory Agents
  • Flavonoids
  • Glucuronates
  • Plant Extracts
  • apigenin-7-O-glucuronide
  • scutellarin
  • Apigenin