Use of an immobilized enzyme reactor for the analysis of residues of 17 alpha-methyltestosterone in trout by high-performance liquid chromatography

J Chromatogr. 1991 Apr 5;564(2):461-7. doi: 10.1016/0378-4347(91)80514-d.

Abstract

We have recently observed in trout that 48 h after ingestion of a single dose of [14C]-17 alpha-methyltestosterone ([14C]-MT), 25% of the radioactivity was still in the carcass, corresponding to metabolites of 17-MT. These compounds have no appreciable chromophore, fluorophore or electrophore, therefore the usual detection systems was not satisfactory for their analysis. Consequently a method was developed for high-performance liquid chromatographic separation and detection of two of the major tissue metabolites of 17-MT: 5 alpha-androstane-17 alpha-methyl-3 alpha,17 beta-diol and 5 beta-androstane-17 alpha-methyl-3 alpha,17 beta-diol. A column of immobilized 3 alpha-hydroxysteroid dehydrogenase was prepared and used for detection. The NADH produced from 3-hydroxysteroids by this immobilized enzyme reactor was monitored fluorimetrically. The detection limit of this method, as obtained from the calibration curve, was at the picomole level; the limit of quantification in muscle was 1 microgram/kg, at a signal-to-noise ratio of 4.

MeSH terms

  • Animals
  • Chromatography, High Pressure Liquid / methods*
  • Enzymes, Immobilized
  • Methyltestosterone / analysis*
  • Methyltestosterone / metabolism
  • Muscles / chemistry
  • Muscles / metabolism
  • Trout / metabolism*

Substances

  • Enzymes, Immobilized
  • Methyltestosterone