Catalytic wet air oxidation of aniline with nanocasted Mn-Ce-oxide catalyst

Environ Sci Technol. 2008 Jul 15;42(14):5165-70. doi: 10.1021/es703070h.

Abstract

The catalytic wet air oxidation of aqueous solution containing 1000 ppm aniline was conducted in a trickle-bed reactor packed with a novel nanocasted Mn-Ce-oxide catalyst (surface area of 300 m2/g) prepared using SBA-15 silica as a hard template. A range of liquid hourly space velocities (5-20 h(-1)) and temperatures (110-140 degrees C) at 10 bar of oxygen were tested. The experiments were conducted to provide the intrinsic performance of the catalysts. Complete aniline conversion, 90% TOC conversion, and 80% nitrogen mineralization were achieved at 140 degrees C and 5 h(-1). Blank experiments yielded relatively low homogeneous aniline (<35%) and negligible TOC conversions. Fast deactivation of the catalysts was experienced due to leaching caused by complexation with aniline. Acidification of the solution with HCI (molar HCI to aniline ratio of 1.2) was necessary to avoid colloidization and leaching of the nanoparticulate catalyst components. The catalyst displayed stable performance for over 200 h on stream.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acids / chemistry
  • Air*
  • Aniline Compounds / chemistry*
  • Catalysis
  • Cesium / chemistry*
  • Manganese / chemistry*
  • Molecular Structure
  • Nanostructures*
  • Nitrogen / chemistry
  • Oxidation-Reduction
  • Silicon Dioxide / chemistry
  • Water / chemistry

Substances

  • Acids
  • Aniline Compounds
  • SBA-15
  • Water
  • Cesium
  • Manganese
  • Silicon Dioxide
  • Nitrogen
  • aniline