Improved synthesis of the epoxy isoprostane phospholipid PEIPC and its reactivity with amines

Org Lett. 2008 Oct 2;10(19):4207-9. doi: 10.1021/ol8014804. Epub 2008 Aug 28.

Abstract

An improved synthesis of the naturally occurring hydroxy ketone 1-palmitoyl-2-(5,6)-epoxyisoprostane E 2- sn-glycero-3-phosphocholine (PEIPC) 1, a compound that plays a role in endothelial activation in atherosclerosis, has been carried out using a PMB ether as the key protecting group. Opening of an intermediate with pentylamine shows that the allylic epoxide is the position of attack by nucleophiles.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Alcohols / chemistry
  • Amines / chemistry*
  • Isoprostanes / chemical synthesis*
  • Isoprostanes / chemistry
  • Phosphatidylcholines / chemical synthesis*
  • Phosphatidylcholines / chemistry

Substances

  • 1-palmitoyl-2-(epoxyisoprostane-E2)-sn-glycero-3-phosphocholine
  • Alcohols
  • Amines
  • Isoprostanes
  • Phosphatidylcholines