Diversity-oriented synthesis of novel polycyclic scaffolds using polymer-bound reagents

Chem Commun (Camb). 2008 Oct 14:(38):4619-21. doi: 10.1039/b807869f. Epub 2008 Jul 28.

Abstract

A concise sequence utilizing a Petasis three component reaction followed by a tandem aza-Cope-Mannich cyclization afforded novel polycyclic heterocycles in good yield; alternative iminium cyclization based on a Pictet-Spengler reaction or aminal formation led to divergent pathways affording skeletal diversity.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aza Compounds / chemistry
  • Cyclization
  • Heterocyclic Compounds / chemical synthesis
  • Indicators and Reagents / chemistry*
  • Mannich Bases / chemistry
  • Polycyclic Compounds / chemical synthesis*
  • Polymers / chemistry*

Substances

  • Aza Compounds
  • Heterocyclic Compounds
  • Indicators and Reagents
  • Mannich Bases
  • Polycyclic Compounds
  • Polymers