Sensitive determination of 20(S)-protopanaxadiol in rat plasma using HPLC-APCI-MS: application of pharmacokinetic study in rats

J Pharm Biomed Anal. 2008 Dec 15;48(5):1476-80. doi: 10.1016/j.jpba.2008.09.045. Epub 2008 Oct 8.

Abstract

20(S)-Protopanaxadiol (PPD), the main metabolite of protopanoxadiol type ginsenosides (e.g. Rg3 and Rh2), is a very promising anti-cancer drug candidate. To evaluate the pharmacokinetic property of PPD, we reported a reliable, sensitive and simple method utilizing liquid chromatography (HPLC)-atmospheric pressure chemical ionization-mass spectrometry (APCI-MS) to determine PPD. PPD and the internal standard, panoxadiol (PD) were extracted from plasma with acetic ether, separated on a C18 reverse column, and then analyzed by APCI-MS. Targeting fragment ion at m/z 425 for both PPD and PD was monitored in selected-ion monitoring (SIM) mode. PPD can be quantitatively determined at the concentration as low as 1 ng/mL using 200 microL plasma. And the sensitive method showed excellent linearity over a range from 1 to 1000 ng/mL, high recovery, accuracy and precision at the concentrations of 2.5, 100.0 and 1000.0 ng/mL, respectively. The method was successfully applied to pharmacokinetic study of PPD in rats. Pharmacokinetic parameters were calculated and absolute bioavailability of PPD was 36.8+/-12.4%, at least ten times higher than that of Rg3 and Rh2, indicating its good absorption in gastrointestinal tract. It was further suggested that PPD be a promising anti-cancer candidate and probably responsible for the observed pharmacological activity of Rg3 and Rh2.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Animals
  • Anticarcinogenic Agents / administration & dosage
  • Anticarcinogenic Agents / chemistry
  • Anticarcinogenic Agents / pharmacokinetics*
  • Area Under Curve
  • Atmospheric Pressure
  • Biological Availability
  • Calibration
  • Chromatography, High Pressure Liquid / methods
  • Guidelines as Topic
  • Half-Life
  • Injections, Intravenous
  • Male
  • Mass Spectrometry / methods*
  • Metabolic Clearance Rate
  • Molecular Structure
  • Quality Control
  • Rats
  • Rats, Sprague-Dawley
  • Reference Standards
  • Reproducibility of Results
  • Sapogenins / administration & dosage
  • Sapogenins / chemistry
  • Sapogenins / pharmacokinetics*
  • Sensitivity and Specificity
  • Spectrometry, Mass, Electrospray Ionization / methods

Substances

  • Anticarcinogenic Agents
  • Sapogenins
  • protopanaxadiol