A comparison of two determination methods for studying degradation kinetics of the major anthocyanins from blood orange

J Agric Food Chem. 2009 Jan 14;57(1):245-9. doi: 10.1021/jf8021964.

Abstract

The thermal degradation of cyanidin 3-(6''-malonyl) glucoside and cyanidin 3-glucoside, which are the two major anthocyanins in blood orange juice, have been investigated using the pH-differential method and RP-HPLC method, respectively. Similar results could be obtained when the degradation kinetics of cyanidin 3-glucoside were studied by either the HPLC method or the pH-differential method. However, contrary results were obtained in the case of cyanidin 3-(6''-malonyl) glucoside. The HPLC analysis indicated that cyanidin 3-(6''-malonyl) glucoside was labile to eliminate a malonyl moiety to form cyanidin 3-glucoside before disappearing during thermal treatment and showed a lower thermal stability than cyanidin 3-glucoside, whereas the result obtained by the pH-differential method actually reflected the content of both cyanidin 3-(6''-malonyl) glucoside and its degradation intermediate. This caused an overestimate of the stability of cyanidin 3-(6''-malonyl) glucoside.

Publication types

  • Comparative Study

MeSH terms

  • Anthocyanins / analysis
  • Anthocyanins / chemistry*
  • Beverages / analysis
  • Chromatography, High Pressure Liquid
  • Citrus sinensis / chemistry*
  • Fruit / chemistry*
  • Glucosides / analysis
  • Glucosides / chemistry
  • Hot Temperature
  • Hydrogen-Ion Concentration
  • Kinetics

Substances

  • Anthocyanins
  • Glucosides
  • cyanidin-3-(6-malonylglucoside)
  • cyanidin-3-O-beta-glucopyranoside