A simple and sensitive HPLC-ESI-MS/MS method for the determination of andrographolide in human plasma

J Chromatogr B Analyt Technol Biomed Life Sci. 2009 Feb 15;877(5-6):502-6. doi: 10.1016/j.jchromb.2008.12.065. Epub 2009 Jan 6.

Abstract

A liquid chromatography-electrospray ionization tandem mass spectrometry (HPLC-ESI-MS/MS) method for the determination of andrographolide in human plasma was established. Dehydroandrographolide was used as the internal standard (I.S.). The plasma samples were deproteinized with methanol and separated on a Hanbon C(18) column with a mobile phase of methanol-water (70:30, v/v). HPLC-ESI-MS/MS was performed in the selected ion monitoring (SIM) mode using target ions at [M-H(2)O-H](-), m/z 331.1 for andrographolide and [M-H](-), m/z 331.1 for the I.S. Calibration curve was linear over the range of 1.0-150.0ng/mL. The chromatographic separation was achieved in less than 6.5min. The lower limits of quantification (LLOQ) was 1.0ng/mL. The intra and inter-run precisions were less than 6.95 and 7.22%, respectively. The method was successfully applied to determine the plasma concentrations of andrographolide in Chinese volunteers.

Publication types

  • Clinical Trial

MeSH terms

  • Anti-Inflammatory Agents / administration & dosage
  • Anti-Inflammatory Agents / blood
  • Anti-Inflammatory Agents / chemistry
  • Anti-Inflammatory Agents / pharmacokinetics
  • Calibration
  • Chromatography, High Pressure Liquid / methods*
  • Diterpenes / administration & dosage
  • Diterpenes / blood*
  • Diterpenes / chemistry
  • Diterpenes / pharmacokinetics
  • Drug Stability
  • Humans
  • Male
  • Reference Standards
  • Reproducibility of Results
  • Spectrometry, Mass, Electrospray Ionization / methods*

Substances

  • Anti-Inflammatory Agents
  • Diterpenes
  • andrographolide
  • dehydroandrographolide