Sequential Cu(I)/Pd(0)-catalyzed multicomponent coupling and annulation protocol for the synthesis of indenoisoquinolines

Org Lett. 2009 Feb 19;11(4):815-8. doi: 10.1021/ol802755z.

Abstract

Copper-catalyzed coupling of imines, vinylstannanes, or alkynes and o-bromoaroyl chlorides followed by Pd(0)-catalyzed annulations afforded indenoisoquinolines. Protocols requiring minimal purifications were developed, providing new methods for the construction of combinatorial libraries.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Alkynes / chemistry*
  • Catalysis
  • Combinatorial Chemistry Techniques
  • Copper / chemistry*
  • Hydrocarbons, Halogenated / chemistry*
  • Imines / chemistry*
  • Indenes / chemical synthesis*
  • Indenes / chemistry
  • Isoquinolines / chemical synthesis*
  • Isoquinolines / chemistry
  • Molecular Structure
  • Palladium / chemistry
  • Tin Compounds / chemistry*
  • Vinyl Compounds / chemistry*

Substances

  • Alkynes
  • Hydrocarbons, Halogenated
  • Imines
  • Indenes
  • Isoquinolines
  • Tin Compounds
  • Vinyl Compounds
  • stannane
  • Palladium
  • Copper