Laser-induced alignment and orientation of quantum-state-selected large molecules

Phys Rev Lett. 2009 Jan 16;102(2):023001. doi: 10.1103/PhysRevLett.102.023001. Epub 2009 Jan 12.

Abstract

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and used as targets for further experiments. As an illustration, we demonstrate an unprecedented degree of laser-induced one-dimensional alignment (cos;(2)theta_(2D)=0.97) and strong orientation of state-selected iodobenzene molecules. This method should enable experiments on pure samples of polar molecules in their rotational ground state, offering new opportunities in molecular science.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Iodobenzenes / chemistry
  • Lasers, Solid-State*
  • Models, Chemical*
  • Peptides / chemistry
  • Quantum Theory*

Substances

  • Iodobenzenes
  • Peptides
  • iodobenzene