Influence of Ca(2+) ions on the activity of lantibiotics containing a mersacidin-like lipid II binding motif

Appl Environ Microbiol. 2009 Jul;75(13):4427-34. doi: 10.1128/AEM.00262-09. Epub 2009 May 8.

Abstract

Mersacidin binds to lipid II and thus blocks the transglycosylation step of the cell wall biosynthesis. Binding of lipid II involves a special motif, the so-called mersacidin-lipid II binding motif, which is conserved in a major subgroup of lantibiotics. We analyzed the role of Ca(2+) ions in the mode of action of mersacidin and some related peptides containing a mersacidin-like lipid II binding motif. We found that the stimulating effect of Ca(2+) ions on the antimicrobial activity known for mersacidin also applies to plantaricin C and lacticin 3147. Ca(2+) ions appear to facilitate the interaction of the lantibiotics with the bacterial membrane and with lipid II rather than being an essential part of a peptide-lipid II complex. In the case of lacticin 481, both the interaction with lipid II and the antimicrobial activity were Ca(2+) independent.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Anti-Bacterial Agents / pharmacology*
  • Bacteriocins / metabolism
  • Bacteriocins / pharmacology*
  • Calcium / pharmacology*
  • Enzyme Activators / pharmacology*
  • Models, Molecular
  • Molecular Sequence Data
  • Peptides / metabolism*
  • Uridine Diphosphate N-Acetylmuramic Acid / analogs & derivatives*
  • Uridine Diphosphate N-Acetylmuramic Acid / metabolism

Substances

  • Anti-Bacterial Agents
  • Bacteriocins
  • Enzyme Activators
  • Peptides
  • Uridine Diphosphate N-Acetylmuramic Acid
  • muramyl-NAc-(pentapeptide)pyrophosphoryl-undecaprenol
  • mersacidin
  • Calcium