Effects of P-glycoprotein and Mrp2 inhibitors on the hepatobiliary disposition of Rhodamine 123 and its glucuronidated metabolite in isolated perfused rat livers

J Pharm Sci. 2010 Jan;99(1):455-66. doi: 10.1002/jps.21831.

Abstract

The hepatobiliary disposition of rhodamine 123 (RH-123) and its glucuronidated (RH-Glu) and deacylated (RH-110) metabolites were studied in an isolated perfused rat liver (IPRL) model in the presence and absence of P-glycoprotein (P-gp) and Mrp2 inhibitors. A single dose (180 microg) of RH-123 was added to a recirculating perfusate in the absence (Control) or presence of cyclosporine A (CyA) or dibromosulfophthalein (DBSP) in the perfusate. Serial (0-90 min) perfusate and bile and terminal liver samples were collected for analysis by HPLC. In the Control livers, 25.4 +/- 2.2% (mean +/- SD) of the dose was recovered as RH-123 (11.7 +/- 2.0%) and RH-Glu (13.2 +/- 0.9%) in the bile. Whereas CyA substantially (90%) reduced (p < 0.001) the biliary excretion of RH-123 without affecting the excretion of RH-Glu, DBSP reduced the biliary excretion of RH-Glu by >80% (p < 0.001) with no effect on the biliary excretion of RH-123. Mass balance studies showed that DBSP, in addition to reducing the biliary clearance of RH-Glu, also strongly inhibited the glucuronidation of RH-123, an effect that was confirmed in vitro using the glucuronidation marker umbelliferone. It is concluded that the use of RH-123 in an IPRL model may serve as a dual marker for the determination of the altered functions of P-gp and/or Mrp2.

MeSH terms

  • ATP Binding Cassette Transporter, Subfamily B, Member 1 / antagonists & inhibitors*
  • ATP Binding Cassette Transporter, Subfamily B, Member 1 / physiology
  • ATP-Binding Cassette Transporters / antagonists & inhibitors*
  • ATP-Binding Cassette Transporters / physiology
  • Animals
  • Biliary Tract / drug effects
  • Biliary Tract / metabolism*
  • Chromatography, High Pressure Liquid
  • Cyclosporine / pharmacology
  • Dose-Response Relationship, Drug
  • Fluorescent Dyes / pharmacokinetics*
  • Glucuronides / metabolism*
  • In Vitro Techniques
  • Liver / drug effects
  • Liver / metabolism*
  • Male
  • Microsomes, Liver / drug effects
  • Microsomes, Liver / metabolism
  • Perfusion
  • Rats
  • Rats, Sprague-Dawley
  • Rhodamine 123 / metabolism
  • Rhodamine 123 / pharmacokinetics*
  • Sulfobromophthalein / pharmacology
  • Time Factors
  • Tissue Distribution

Substances

  • ATP Binding Cassette Transporter, Subfamily B, Member 1
  • ATP-Binding Cassette Transporters
  • Abcc2 protein, rat
  • Fluorescent Dyes
  • Glucuronides
  • Sulfobromophthalein
  • dibromosulphthalein
  • Rhodamine 123
  • Cyclosporine