Relative stereochemical determination and synthesis of the C1-C17 fragment of a new natural polyketide

J Org Chem. 2009 Sep 18;74(18):7034-45. doi: 10.1021/jo9012833.

Abstract

The challenging determination of the relative stereochemistry of a complex natural polyketide portion was achieved. After careful NMR analysis, a concise synthesis of a set of possible relative diastereomers (only 6 diastereomers out of the 32 initially envisioned) has been carried out using a common strategy based on enantioselective aldol reactions. With a high predictability, final NMR comparison established the relative stereochemistry of the C1-C17 fragment of this natural product.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biological Products* / chemical synthesis
  • Biological Products* / chemistry
  • Macrolides* / chemical synthesis
  • Macrolides* / chemistry
  • Magnetic Resonance Spectroscopy
  • Stereoisomerism

Substances

  • Biological Products
  • Macrolides