Rectification of the ionic current through carbon nanotubes by electrostatic assembly of polyelectrolytes

Nano Lett. 2009 Nov;9(11):3853-9. doi: 10.1021/nl9020683.

Abstract

Rectification of the ionic current flowing through nanotubes embedded in a polymeric membrane is achieved by selective adsorption of polycations to the nanotubes' mouths. A one-dimensional model of ionic flux through a nanotube with charged entrance regions qualitatively describes current-voltage curves before and after polycation exposure; reversal potential measurements confirm that charge reversal takes place upon polycation adsorption. The inherent simply of this electrostatic approach makes it attractive in membrane and nanofluidic applications employing rectification.