DNA aptamer-micelle as an efficient detection/delivery vehicle toward cancer cells

Proc Natl Acad Sci U S A. 2010 Jan 5;107(1):5-10. doi: 10.1073/pnas.0909611107. Epub 2009 Dec 22.

Abstract

We report the design of a self-assembled aptamer-micelle nanostructure that achieves selective and strong binding of otherwise low-affinity aptamers at physiological conditions. Specific recognition ability is directly built into the nanostructures. The attachment of a lipid tail onto the end of nucleic acid aptamers provides these unique nanostructures with an internalization pathway. Other merits include: extremely low off rate once bound with target cells, rapid recognition ability with enhanced sensitivity, low critical micelle concentration values, and dual-drug delivery pathways. To prove the potential detection/delivery application of this aptamer-micelle in biological living systems, we mimicked a tumor site in the blood stream by immobilizing tumor cells onto the surface of a flow channel device. Flushing the aptamer-micelles through the channel demonstrated their selective recognition ability under flow circulation in human whole-blood sample. The aptamer-micelles show great dynamic specificity in flow channel systems that mimic drug delivery in the blood system. Therefore, our DNA aptamer-micelle assembly has shown high potential for cancer cell recognition and for in vivo drug delivery applications.

Publication types

  • Evaluation Study
  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Aptamers, Nucleotide* / chemistry
  • Aptamers, Nucleotide* / metabolism
  • Aptamers, Nucleotide* / therapeutic use
  • Cell Line, Tumor
  • Drug Carriers / chemistry
  • Drug Carriers / metabolism
  • Drug Delivery Systems*
  • Endocytosis
  • Flow Cytometry / methods
  • Fluorescent Dyes / metabolism
  • Humans
  • Micelles*
  • Nanostructures / chemistry*
  • Neoplasms / drug therapy*

Substances

  • Aptamers, Nucleotide
  • Drug Carriers
  • Fluorescent Dyes
  • Micelles