Determining the morphology of polystyrene-block-poly(2-vinylpyridine) micellar reactors for ZnO nanoparticle synthesis

Langmuir. 2010 May 18;26(10):7431-6. doi: 10.1021/la904143f.

Abstract

We report the use of reverse PS-b-P2VP diblock copolymer micelles as true nanoscale-sized reactor vessels to synthesize ZnO nanoparticles. The reverse micelles were formed in toluene and then sequentially loaded with zinc acetate dihydrate and tetramethylammonium hydroxide reactants. Moreover, high spatial resolution Z-contrast imaging and EDX spectroscopy techniques were used to confirm the segregation of the Zn cation to the core of the loaded micelles. Determining the chemical distribution with high nanoscale spatial resolution is shown to complement the less direct characterization by AFM, DLS and FTIR, thus demonstrating broader implications for the characterization of hybrid nanocomposite systems.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Micelles
  • Nanoparticles / chemistry*
  • Particle Size
  • Polystyrenes / chemistry*
  • Polyvinyls / chemistry*
  • Surface Properties
  • Zinc Oxide / chemical synthesis*
  • Zinc Oxide / chemistry

Substances

  • Micelles
  • Polystyrenes
  • Polyvinyls
  • poly(styrene)-block-poly(2-vinylpyrindine) diblock copolymer
  • Zinc Oxide