ESI FTICR-MS analysis of larvae from the marine sponge Luffariella variabilis

Mar Drugs. 2010 Jan 22;8(1):190-9. doi: 10.3390/md8010190.

Abstract

The viviparous Great Barrier Reef sponge Luffariella variabilis (Poléjaeff 1884) contains a range of secondary metabolites, including manoalide (1) and manoalide monoacetate (3). ESI (+) FTICR-MS accurate mass determination has, for the first time, been used to detected the presence of 3 only in an organic extract of a single L. variabilis larva showing that the parentally produced 3 is sequestered in the larva. As 3 has previously been shown to have antibacterial and quorum sensing inhibition activity, and readily converts to 1, which also exhibits similar activity, it may provide a chemical defence against predation and microbial attack.

Keywords: ESI FTICR-MS; Luffariella variabilis; constitutive defence; larvae; manoalide monoacetate.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetates / analysis*
  • Acetates / chemistry
  • Analytic Sample Preparation Methods
  • Animals
  • Anti-Bacterial Agents / analysis
  • Anti-Bacterial Agents / chemistry
  • Larva / chemistry
  • Marine Toxins / analysis
  • Marine Toxins / chemistry
  • Microchemistry / methods
  • Molecular Structure
  • Pacific Ocean
  • Porifera / chemistry*
  • Queensland
  • Spectrometry, Mass, Electrospray Ionization / methods*
  • Spectroscopy, Fourier Transform Infrared / methods*
  • Terpenes / analysis*
  • Terpenes / chemistry

Substances

  • Acetates
  • Anti-Bacterial Agents
  • Marine Toxins
  • Terpenes
  • manoalide