Transformation and sorption of the veterinary antibiotic sulfadiazine in two soils: a short-term batch study

Environ Sci Technol. 2010 Jun 15;44(12):4651-7. doi: 10.1021/es100141m.

Abstract

The worldwide use of veterinary antibiotics poses a continuous threat to the environment. There is, however, a lack of mechanistic studies on sorption and transformation processes for environmental assessment in soils. Two-week batch sorption experiments were performed with the antibiotic sulfadiazine (SDZ) in the plow layer and the subsoil of a loamy sand and a silty loam. The sorption and transformation parameters of SDZ and its main transformation products N1-2-(4-hydroxypyrimidinyl) benzenesulfanilamide (4-OH-SDZ) and 4-(2-iminopyrimidin-1(2H)-yl)aniline (An-SDZ) were estimated using a global optimization algorithm. A two-stage, one-rate sorption model combined with a first-order transformation model adequately described the batch data. Sorption of SDZ was nonlinear, time-dependent, and affected by pH, with a higher sorption capacity for the loamy sand. Transformation of SDZ into 4-OH-SDZ occurred only in the liquid phase, with half-life values of 1 month in the plow layers and 6 months in the subsoils. Under the exclusion of light, An-SDZ was formed in substantial amounts in the silty loam only, with liquid phase half-life values of 2 to 3 weeks. Despite the rather large parameter uncertainties, which may be reduced using additional information obtained from sequential solid phase extraction, the proposed method provides a framework to assess the fate of antibiotics in soils.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adsorption
  • Biodegradation, Environmental
  • Biotransformation
  • Carbon Radioisotopes
  • Environmental Restoration and Remediation / methods*
  • Kinetics
  • Models, Chemical
  • Soil / analysis*
  • Sulfadiazine / chemistry
  • Sulfadiazine / isolation & purification*
  • Sulfadiazine / metabolism*
  • Time Factors
  • Veterinary Drugs / chemistry
  • Veterinary Drugs / isolation & purification*
  • Veterinary Drugs / metabolism*

Substances

  • Carbon Radioisotopes
  • Soil
  • Veterinary Drugs
  • Sulfadiazine