A silicon nanowire-based electrochemical glucose biosensor with high electrocatalytic activity and sensitivity

Nanoscale. 2010 Sep;2(9):1704-7. doi: 10.1039/c0nr00314j. Epub 2010 Aug 5.

Abstract

An electrochemical glucose biosensor was developed by immobilizing glucose oxidase (GOx) on an electrode decorated with a novel nanostructure, silicon nanowires (SiNWs) with in situ grown gold nanoparticles (AuNPs). The immobilized GOx displayed a pair of well-defined and quasi-reversible redox peaks with a formal potential (E(o ')) of -0.376 V in a phosphate buffer solution. The fabricated glucose biosensor has good electrocatalytic activity toward oxidation of glucose. In addition, such resultant SiNWs-based glucose biosensor possesses high biological affinity. Particularly, the apparent Michaelis-Mentan constant was estimated to be 0.902 mM, which is much smaller than the reported values for GOx at a range of nanomaterials-incorporated electrodes. Consequently, this novel SiNWs-based biosensor is expected to be a promising tool for biological assays (e.g., monitoring blood glucose).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biocatalysis
  • Biosensing Techniques / methods*
  • Electrochemical Techniques / methods*
  • Electrodes
  • Enzymes, Immobilized / chemistry
  • Enzymes, Immobilized / metabolism
  • Glucose / analysis*
  • Glucose Oxidase / chemistry
  • Glucose Oxidase / metabolism
  • Gold / chemistry
  • Metal Nanoparticles / chemistry
  • Nanowires / chemistry*
  • Nanowires / ultrastructure
  • Silicon / chemistry*

Substances

  • Enzymes, Immobilized
  • Gold
  • Glucose Oxidase
  • Glucose
  • Silicon