Catalytic digestion of human tumor necrosis factor-α by antibody heavy chain

FEBS J. 2010 Sep;277(18):3823-32. doi: 10.1111/j.1742-4658.2010.07785.x. Epub 2010 Aug 16.

Abstract

It has long been an important task to prepare a catalytic antibody capable of digesting a targeting crucial protein that controls specific life functions. Tumor necrosis factor-α (TNF-α) is a cytokine and an important molecule concerned with autoimmune diseases such as rheumatoid arthritis, chronic obstructive pulmonary disease, and Crohn's disease. A mAb (ETNF-6 mAb) raised against human TNF-α was prepared, and the steric conformation was created by using molecular modeling after the cDNA was sequenced. The heavy chain (ETNF-6-H) of the mAb was considered to possess a catalytic triad-like structure in the complementarity determining regions (CDRs). As a result, ETNF-6-H exhibited a peptidase and a protease activity. In fact, ETNF-6-H predominantly cleaved the Ser5-Arg6 bond of TNF-α at the first step, resulting in the generation of a fragment of ∼ 17 kDa. This fragment was digested to a smaller molecule of 15 kDa by scission of the Gln21-Ala22 bond. The intermediate product was further converted into a fragment of 13.3 kDa by successive cleavage of the Leu36-Leu37 and Asn39-Gly40 bonds. The heavy chain possessed a protease activity against TNF-α with a multicleavage site.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Antibodies, Catalytic / chemistry
  • Antibodies, Catalytic / immunology
  • Antibodies, Catalytic / isolation & purification
  • Antibodies, Catalytic / metabolism*
  • Antibodies, Monoclonal / chemistry
  • Antibodies, Monoclonal / immunology*
  • Antibodies, Monoclonal / isolation & purification
  • Antibodies, Monoclonal / metabolism*
  • Antibody Affinity
  • Base Sequence
  • Biocatalysis
  • Cross Reactions
  • Female
  • Humans
  • Hydrolysis
  • Immunoglobulin Heavy Chains / chemistry
  • Immunoglobulin Heavy Chains / immunology
  • Immunoglobulin Heavy Chains / isolation & purification
  • Immunoglobulin Heavy Chains / metabolism*
  • Kinetics
  • Mice
  • Mice, Inbred BALB C
  • Molecular Sequence Data
  • Peptides / chemistry
  • Peptides / metabolism
  • Protein Conformation
  • Substrate Specificity
  • Tumor Necrosis Factor-alpha / immunology*
  • Tumor Necrosis Factor-alpha / metabolism*

Substances

  • Antibodies, Catalytic
  • Antibodies, Monoclonal
  • Immunoglobulin Heavy Chains
  • Peptides
  • Tumor Necrosis Factor-alpha