A bismuth(III)-catalyzed Friedel-Crafts cyclization and stereocontrolled organocatalytic approach to (-)-platensimycin

Org Lett. 2010 Dec 3;12(23):5510-3. doi: 10.1021/ol102390t. Epub 2010 Oct 29.

Abstract

A high yielding route to the (-)-platensimycin core is communicated. This entailed the discovery of Bi(OTf)(3) to catalyze a Friedel-Crafts cyclization of a free lactol, supplemented by LiClO(4) to suppress the Lewis basicity of the sulfonate group. After TBAF-promoted cyclodearomatization, a diastereoselective conjugate reduction of a dienone was achieved by adopting amine-based organocatalytic rationales to reverse the inherent steric control of the substrate.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adamantane / chemistry*
  • Aminobenzoates / chemistry*
  • Anilides / chemistry*
  • Bismuth / chemistry*
  • Catalysis
  • Cyclization
  • Molecular Structure
  • Stereoisomerism

Substances

  • Aminobenzoates
  • Anilides
  • Adamantane
  • platensimycin
  • Bismuth