Labelling of histone H5 and its interaction with DNA. 1. Histone H5 labelling with fluorescein isothiocyanate

J Biomol Struct Dyn. 1990 Jun;7(6):1291-300. doi: 10.1080/07391102.1990.10508566.

Abstract

Histone H5 has been labelled with fluorescein isothiocyanate (FITC) with particular attention to the reaction conditions (pH, reaction time and input FITC/H5 molar ratio) and to the complete elimination of non-covalently bound dye. We preferred to use reaction conditions which yielded non-specific uniform labelling rather than specific alpha-NH2 terminal labelling, in order to obtain higher sensitivity in further studies dealing with the detection of perturbation at the binding sites of H5 on DNA. FITC-labelled H5 was further characterized by absorption and circular dichroism spectroscopy, and the fluorescein probe titrated in the 4-8 pH range. The structural integrity of H5 was found to be preserved after labelling. The positive electrostatic potential of the environment in which the FITC probe is embedded in the arginine/lysine-rich tails of H5 is believed to be responsible for the drop of pK of 1 unit found for H5-FITC as compared to free FITC. For the globular part of H5, the pK of covalently-bound FITC was only slightly lowered; this is a consequence of the much lower content in positively-charged amino-acid side chains in this region.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Chickens
  • Circular Dichroism
  • DNA / metabolism*
  • Electrophoresis, Polyacrylamide Gel
  • Fluorescein-5-isothiocyanate
  • Fluoresceins*
  • Fluorescent Dyes*
  • Histones / metabolism*
  • Hydrogen-Ion Concentration
  • Thiocyanates*
  • Time Factors

Substances

  • Fluoresceins
  • Fluorescent Dyes
  • Histones
  • Thiocyanates
  • DNA
  • Fluorescein-5-isothiocyanate