Determination of tryptophan and kynurenine in human plasma by liquid chromatography-electrochemical detection with multi-wall carbon nanotube-modified glassy carbon electrode

Biomed Chromatogr. 2011 Aug;25(8):938-42. doi: 10.1002/bmc.1550. Epub 2010 Dec 10.

Abstract

A novel method was developed for the simultaneous determination of kynurenine and tryptophan by high-performance liquid chromatography with electrochemical detection at multi-wall carbon nanotube (MWCNT)-modified glassy carbon electrode. The separation and detection conditions were optimized. The typical HPLC experiments were conducted by using a reversed-phase ODS column with a mobile phase consisting of stock acetate buffer (pH 5)-methanol (4:1, v/v) using an isocratic elution at the flow rate of 1.0 mL/min. The obtained LODs for kynurenine and tryptophane were 0.5 and 0.4 µmol/L, respectively. The analytical method for human plasma samples was validated and confirmed by LC-UV and LC-MS. The recoveries were in the range of 84.8-110%, and the precision was lower than 5.9%.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, High Pressure Liquid / instrumentation*
  • Chromatography, High Pressure Liquid / methods
  • Electrochemical Techniques / instrumentation*
  • Electrochemical Techniques / methods
  • Electrodes
  • Humans
  • Kynurenine / blood*
  • Nanotubes, Carbon / chemistry*
  • Reproducibility of Results
  • Tryptophan / blood*

Substances

  • Nanotubes, Carbon
  • Kynurenine
  • Tryptophan