Enhancement of single-molecule fluorescence signals by colloidal silver nanoparticles in studies of protein translation

ACS Nano. 2011 Jan 25;5(1):399-407. doi: 10.1021/nn101839t. Epub 2010 Dec 16.

Abstract

Metal-enhanced fluorescence (MEF) increased total photon emission of Cy3- and Cy5-labeled ribosomal initiation complexes near 50 nm silver particles 4- and 5.5-fold, respectively. Fluorescence intensity fluctuations above shot noise, at 0.1-5 Hz, were greater on silver particles. Overall signal-to-noise ratio was similar or slightly improved near the particles. Proximity to silver particles did not compromise ribosome function, as measured by codon-dependent binding of fluorescent tRNA, dynamics of fluorescence resonance energy transfer between adjacent tRNAs in the ribosome, and tRNA translocation induced by elongation factor G.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Base Sequence
  • Carbocyanines / chemistry
  • Colloids
  • Fluorescence Resonance Energy Transfer*
  • Metal Nanoparticles / chemistry*
  • Photobleaching
  • Photons
  • Protein Biosynthesis*
  • RNA, Messenger / genetics
  • RNA, Transfer / genetics
  • RNA, Transfer / metabolism
  • Ribosomes / metabolism
  • Silver / chemistry*

Substances

  • Carbocyanines
  • Colloids
  • RNA, Messenger
  • cyanine dye 3
  • cyanine dye 5
  • Silver
  • RNA, Transfer