Preparation and characterization of chitosan-grafted-poly(2-amino-4,5-pentamethylene-thiophene-3-carboxylic acid N'-acryloyl-hydrazide) chelating resin for removal of Cu(II), Co(II) and Ni(II) metal ions from aqueous solutions

Int J Biol Macromol. 2011 May 1;48(4):558-65. doi: 10.1016/j.ijbiomac.2011.01.018. Epub 2011 Jan 28.

Abstract

The graft copolymerization of ethylacrylate (EA) onto chitosan initiated by potassium persulphate and Mohr's salt combined redox initiator system in limited aqueous medium was carried out in heterogeneous media. Moreover, modification of the grafted chitosan was carried out by reaction of the ester group (-COOEt) with 2-amino-4,5-pentamethylene-thiophene-3-carboxylic acid hydrazide which eventually produce chitosan-grafted-poly(2-amino-4,5-pentamethylene-thiophene-3-carboxylic acid N'-acryloyl-hydrazide) (chitosan-g-ATAH) chelating resin. The application of the modified resin for metal ion uptake was studied using Cu(2+), Co(2+) and Ni(2+) ions. The modified chelating resins were characterized using FTIR spectroscopy, SEM and X-ray diffraction.

MeSH terms

  • Acrylic Resins / chemistry
  • Cation Exchange Resins / chemical synthesis*
  • Cation Exchange Resins / chemistry*
  • Chelating Agents / chemistry*
  • Chitosan / chemistry*
  • Hydrogen-Ion Concentration
  • Metals, Heavy / isolation & purification*
  • Microscopy, Electron, Scanning
  • Molecular Structure
  • Spectrophotometry, Infrared
  • Temperature
  • Time Factors
  • Water Pollutants, Chemical / isolation & purification*
  • Water Purification / methods*
  • X-Ray Diffraction

Substances

  • Acrylic Resins
  • Cation Exchange Resins
  • Chelating Agents
  • Metals, Heavy
  • Water Pollutants, Chemical
  • poly(ethylacrylate)
  • Chitosan