An approach to speed up the isolation of hydrophilic metabolites from natural sources at semipreparative level by using a hydrophilic-lipophilic balance/mixed-mode strong cation exchange-high-performance liquid chromatography/mass spectrometry system

J Chromatogr A. 2011 Apr 1;1218(13):1790-4. doi: 10.1016/j.chroma.2011.01.072. Epub 2011 Jan 31.

Abstract

An approach to speed up the isolation of hydrophilic metabolites in complex natural matrixes by using a HLB/MCX-HPLC/MS system based on the retention properties of hydrophilic-lipophilic and cation exchange polymeric cartridges was developed. This methodology was successfully applied to the re-isolation of small water soluble compounds with completely different structures from two different natural extracts such as a dipeptide (vanchrobactin) from a bacterium culture broth and a pyrrolidine bearing a carboxylic acid moiety (clionapyrrolidine A) from a sponge. This method improved not only the efficiency of the isolation methodology but also the isolation time in relation to the existing methods.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cations / chemistry
  • Chromatography, High Pressure Liquid / methods*
  • Chromatography, Ion Exchange / methods*
  • Complex Mixtures / chemistry*
  • Hydrophobic and Hydrophilic Interactions
  • Mass Spectrometry / methods*
  • Peptides / isolation & purification
  • Porifera
  • Pyrrolidines / isolation & purification
  • Siderophores / isolation & purification*
  • Vibrio
  • Water

Substances

  • Cations
  • Complex Mixtures
  • Peptides
  • Pyrrolidines
  • Siderophores
  • clionapyrrolidine A
  • vanchrobactin
  • Water