The thienotriazolodiazepine Ro 11-1464 increases plasma apoA-I and promotes reverse cholesterol transport in human apoA-I transgenic mice

Br J Pharmacol. 2011 Nov;164(6):1642-51. doi: 10.1111/j.1476-5381.2011.01376.x.

Abstract

Background and purpose: Ro 11-1464 is a thienotriazolodiazepine previously described to selectively stimulate apolipoprotein A-I (apoA-I) production and mRNA level in human liver cells. Here, we studied its effects upon oral administration to human apoA-I transgenic (hapoA-I) mice.

Experimental approach: HapoA-I mice were treated for 5 days with increasing doses of Ro 11-1464. Macrophage reverse cholesterol transport (mph-RCT) was assessed by following [(3) H]-cholesterol mobilization from pre-labelled i.p. injected J774 macrophages to plasma, liver and faeces. Effects on plasma lipids, apoproteins, lecithin-cholesterol : acyltransferase (LCAT) and liver enzymes, as well as on faecal excretion of cholesterol and bile salts, and on liver lipids and mRNA contents were determined.

Key results: Treatment with Ro 11-1464 300 mg·kg(-1) ·day(-1) resulted in a nearly 2-fold increase in plasma apoA-I, a 2- to 3-fold increase in the level of large sized-pre-β high-density lipoprotein and a 3-fold selective up-regulation of hepatic apoA-I mRNA, but a marked decrease in all plasma lipids and LCAT activity. Mpm-RCT was decreased in blood but markedly increased in faecal sterols (4-fold) and bile acids (1.7-fold). However, liver weight and liver enzymes in plasma were also increased, in parallel with an increase in liver cholesterol ester content (all these effect being significant).

Conclusion and implications: In this model Ro 11-1464 causes increased hepatic expression and plasma levels of apoA-I and a suppression of LCAT, and a marked enhancement of reverse cholesterol transport, but also some symptoms of liver toxicity. The compound may therefore be a prototype for a next generation of anti-atherosclerotic medicines.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alanine Transaminase / metabolism
  • Alkaline Phosphatase / metabolism
  • Animals
  • Apolipoprotein A-I / biosynthesis*
  • Apolipoprotein A-I / blood
  • Apolipoprotein A-I / genetics
  • Atherosclerosis / metabolism
  • Azepines / pharmacology*
  • Cholesterol / blood
  • Cholesterol / metabolism*
  • Feces / chemistry
  • Gene Expression Regulation / drug effects
  • Hepatocytes / drug effects
  • Hepatocytes / metabolism
  • Humans
  • Lipid Metabolism / drug effects
  • Lipids / blood*
  • Liver / drug effects
  • Liver / metabolism
  • Liver / pathology
  • Macrophages / metabolism
  • Male
  • Mice
  • Mice, Transgenic
  • Organ Size / drug effects
  • Phosphatidylcholine-Sterol O-Acyltransferase / blood*
  • Thiophenes / pharmacology*

Substances

  • 9-methyl-4-phenyl-6H-thieno(3,2-f)(1,2,4)triazolo(4,3-a)(1,4)diazepine
  • APOA1 protein, human
  • Apolipoprotein A-I
  • Azepines
  • Lipids
  • Thiophenes
  • Cholesterol
  • Phosphatidylcholine-Sterol O-Acyltransferase
  • Alanine Transaminase
  • Alkaline Phosphatase