Palladium catalyzed alkoxy- and aminocarbonylation of vinyl tosylates

Org Lett. 2011 May 6;13(9):2495-7. doi: 10.1021/ol200744s. Epub 2011 Apr 13.

Abstract

The palladium catalyzed alkoxycarbonylation and aminocarbonylation of vinyl tosylates are described. A variety of ketone and aldehyde derived vinyl tosylates may be carbonylated in the presence of primary, secondary, and tertiary alcohols, or primary and secondary amines, to provide the corresponding esters and amides in good yields. The alkoxycarbonylation was applied to a short synthesis of isoguvacine.

MeSH terms

  • Alcohols / chemistry*
  • Amination
  • Anions / chemistry
  • Catalysis
  • Free Radicals / chemistry
  • Ligands
  • Molecular Structure
  • Palladium / chemistry*
  • Vinyl Compounds / chemistry*

Substances

  • Alcohols
  • Anions
  • Free Radicals
  • Ligands
  • Vinyl Compounds
  • alkoxyl radical
  • Palladium