A residue W756 in the P-loop segment of the sodium channel is critical for primaquine binding

Eur J Pharmacol. 2011 Aug 1;663(1-3):1-8. doi: 10.1016/j.ejphar.2011.04.025. Epub 2011 Apr 27.

Abstract

Our study on the wild-type and mutants of the voltage-dependent sodium channel in the rat skeletal muscle Na(v) 1.4 was to examine the possible binding site of primaquine PQ by using an experimental approach. We used a standard voltage-clamp in oocytes. Previously, we had demonstrated that PQ blocks the voltage-dependent sodium current in rat myocytes and that this blocking is concentration-dependent and voltage-independent. The direct-site mutagenesis in the P-loop segment W402C, W756C, W1239C, W1531A at the outer tryptophan-rich lip, and D400C, E758C, K1237C, A1529C of the DEKA locus helped us to identify residues playing a key role in aminoquinoline binding. In full agreement with our computed results, where a 1000-fold reduction of inhibition was measured, the tryptophan 756 is crucial for the reversible modulating effects of PQ. The W756C decreased the blocking effect of PQ in voltage-clamp assays. This new binding site may be important to the development of new drugs that modulate sodium inward currents.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Binding Sites
  • Female
  • Models, Molecular
  • Mutagenesis, Site-Directed
  • Primaquine / metabolism*
  • Protein Binding
  • Protein Structure, Tertiary
  • Rats
  • Sodium Channels / chemistry*
  • Sodium Channels / genetics
  • Sodium Channels / metabolism*
  • Substrate Specificity
  • Tryptophan*

Substances

  • Sodium Channels
  • Tryptophan
  • Primaquine