Highly diastereo- and enantioselective synthesis of syn-β-substituted tryptophans via asymmetric Michael addition of a chiral equivalent of nucleophilic glycine and sulfonylindoles

Chem Commun (Camb). 2011 Aug 7;47(29):8355-7. doi: 10.1039/c1cc12619a. Epub 2011 Jun 21.

Abstract

The asymmetric synthesis of syn-β-substituted tryptophan derivatives was carried out by the Michael addition of chiral equivalent of nucleophilic glycine with sulfonylindoles, and high diastereo- and enantioselectivities were achieved. The resulting adducts were readily converted to syn-β-substituted tryptophans in 96% yield, indicating that the proposed method is a highly efficient route to chiral syn-β-substituted tryptophans.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Coordination Complexes / chemistry
  • Glycine / chemistry*
  • Indoles / chemistry*
  • Nickel / chemistry
  • Schiff Bases / chemistry
  • Stereoisomerism
  • Sulfones / chemistry
  • Tryptophan / chemical synthesis
  • Tryptophan / chemistry*

Substances

  • Coordination Complexes
  • Indoles
  • Schiff Bases
  • Sulfones
  • Nickel
  • indole
  • Tryptophan
  • Glycine