Liquid-gated ambipolar transport in ultrathin films of a topological insulator Bi2Te3

Nano Lett. 2011 Jul 13;11(7):2601-5. doi: 10.1021/nl201561u. Epub 2011 Jun 27.

Abstract

Using ionic-liquid (IL) gating in electric-double-layer transistors (EDLTs), we investigate field-effect electrical transport properties of ultrathin epitaxial films of a topological insulator (TI), Bi(2)Te(3). Because of their extreme thinness, the Bi(2)Te(3) films show a band gap opening and resulting semiconducting transport properties. Near room temperature, an obvious ambipolar transistor operation with an ON-OFF ratio close to 10(3) was observed in the transfer characteristics of liquid-gated EDLTs and further confirmed by a sign change of the Hall coefficients. Modulation of the electronic states and a phase transition from a semiconducting conduction (dR(xx)/dT < 0) to a metallic transport (dR(xx)/dT > 0) were observed in the temperature-dependent resistance of the ultrathin Bi(2)Te(3) channel, demonstrating that the liquid gating is an effective way to modulate the electronic states of TIs.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bismuth / chemistry*
  • Ionic Liquids / chemistry*
  • Membranes, Artificial*
  • Nanotechnology
  • Particle Size
  • Surface Properties
  • Tellurium / chemistry*
  • Temperature
  • Transistors, Electronic*

Substances

  • Ionic Liquids
  • Membranes, Artificial
  • bismuth telluride
  • Tellurium
  • Bismuth