Amide H/D exchange in the thermal transition of bovine pancreatic ribonuclease A

Biochem Biophys Res Commun. 1990 Oct 30;172(2):800-3. doi: 10.1016/0006-291x(90)90745-9.

Abstract

The H/D exchange behavior of RNase A at pH 2.5 at a number of temperatures spanning the thermal transition region has been examined by NMR spectroscopy. The amide proton of V116 has a slow rate of H/D exchange even at temperatures above the midpoint of the thermal transition. The H/D exchange behavior of the peptide corresponding to residues 105-124 of RNase A and the peptide corresponding to residues 115-117 is compared with that of RNase A, showing that folding/unfolding cannot be described by a two-state model, and that both short- and long-range interactions are responsible for the slow rate of H/D exchange.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amides
  • Amino Acid Sequence
  • Animals
  • Cattle
  • Deuterium
  • Hydrogen*
  • Magnetic Resonance Spectroscopy
  • Molecular Sequence Data
  • Oligopeptides / chemical synthesis
  • Pancreas / enzymology
  • Protons
  • Ribonuclease, Pancreatic / metabolism*

Substances

  • Amides
  • Oligopeptides
  • Protons
  • Hydrogen
  • Deuterium
  • Ribonuclease, Pancreatic