Efficient light-harvesting antenna with a multi-porphyrin cascade

J Am Chem Soc. 2011 Aug 31;133(34):13276-9. doi: 10.1021/ja2050343. Epub 2011 Aug 8.

Abstract

A light-harvesting antenna 1 comprising three varieties of porphyrins, each having a different number of ethynyl groups at its meso positions, was designed and synthesized. Antenna 1 exhibits intense absorption throughout the visible region up to 700 nm. Steady-state and time-resolved fluorescence studies showed that singlet-excited-state energy transfer occurs from the peripheral porphyrins to the central porphyrin with >90% efficiency and rate constants on the order of 10(10) s(-1).