Short hydrogen bond between redox-active tyrosine Y(Z) and D1-His190 in the photosystem II crystal structure

Biochemistry. 2011 Nov 15;50(45):9836-44. doi: 10.1021/bi201366j. Epub 2011 Oct 20.

Abstract

The crystal structure of photosystem II (PSII) analyzed at a resolution of 1.9 Å revealed a remarkably short H-bond between redox-active tyrosine Y(Z) and D1-His190 (2.46 Å donor-acceptor distance). Using large-scale quantum mechanical/molecular mechanical (QM/MM) calculations with the explicit PSII protein environment, we were able to reproduce this remarkably short H-bond in the original geometry of the crystal structure in the neutral [Y(Z)O···H···N(ε)-His-N(δ)H···O═Asn] state, but not in the oxidized states, indicating that the neutral state was the one observed in the crystal structure. In addition to the appropriate redox/protonation state of Y(Z) and D1-His190, we found that the presence of a cluster of water molecules played a key role in shortening the distance between Y(Z) and D1-His190. The orientations of the water molecules in the cluster were energetically stabilized by the highly polarized PSII protein environment, where the Ca ion of the oxygen-evolving complex (OEC) and the OEC ligand D1-Glu189 were also involved.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacterial Proteins / chemistry
  • Crystallography, X-Ray
  • Cyanobacteria / chemistry
  • Hydrogen Bonding
  • Models, Molecular
  • Oxidation-Reduction
  • Photosystem II Protein Complex / chemistry*
  • Protons
  • Thermodynamics
  • Tyrosine / chemistry
  • Water / chemistry

Substances

  • Bacterial Proteins
  • Photosystem II Protein Complex
  • Protons
  • Water
  • Tyrosine