Triple ionization of CO2 by valence and inner shell photoionization

J Chem Phys. 2011 Oct 7;135(13):134309. doi: 10.1063/1.3643121.

Abstract

Spectra of triply ionized CO(2) have been obtained from photoionization of the molecule using soft x-ray synchrotron light and an efficient multi-electron coincidence technique. Although all states of the CO(2) (+++) trication are unstable, the ionization energy for formation of molecular ions at a geometry similar to that of the neutral molecule is determined as 74 ± 0.5 eV.