Electropolymerized network of polyamidoamine dendron-coated gold nanoparticles as novel nanostructured electrode surface for biosensor construction

Analyst. 2012 Jan 21;137(2):342-8. doi: 10.1039/c1an15850c. Epub 2011 Nov 24.

Abstract

Polyfuntionalized gold nanoparticles were prepared by using 2-mercaptoethanesulfonic acid, p-aminothiophenol and cysteamine core polyamidoamine G-4 dendron as capping ligands. The nanoparticles were electropolymerized on a Au electrode surface through the formation of a bisaniline-cross-linked network. The enzyme tyrosinase was further crosslinked on this nanostructured matrix. The enzyme electrode, poised at -100 mV, was used for the amperometric quantification of cathecol. The biosensor showed a linear response from 50 nM to 10 μM cathecol, with a low detection limit of 20 nM and a sensitivity of 1.94 A M(-1) cm(2). The electrode retained 96% and 67% of its initial activity after 16 and 30 days of storage at 4 °C under dry conditions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biocompatible Materials / chemistry
  • Biosensing Techniques*
  • Dendrimers / chemistry*
  • Electrochemistry*
  • Electrodes*
  • Enzymes, Immobilized
  • Gold / chemistry*
  • Metal Nanoparticles / chemistry*
  • Monophenol Monooxygenase / chemistry
  • Monophenol Monooxygenase / metabolism
  • Nanostructures / chemistry*

Substances

  • Biocompatible Materials
  • Dendrimers
  • Enzymes, Immobilized
  • PAMAM Starburst
  • Gold
  • Monophenol Monooxygenase