Broadband light management using low-Q whispering gallery modes in spherical nanoshells

Nat Commun. 2012 Feb 7:3:664. doi: 10.1038/ncomms1664.

Abstract

Light trapping across a wide band of frequencies is important for applications such as solar cells and photodetectors. Here, we demonstrate a new approach to light management by forming whispering-gallery resonant modes inside a spherical nanoshell structure. The geometry of the structure gives rise to a low quality-factor, facilitating the coupling of light into the resonant modes and substantial enhancement of the light path in the active material, thus dramatically improving absorption. Using nanocrystalline silicon (nc-Si) as a model system, we observe broadband absorption enhancement across a large range of incident angles. The absorption of a single layer of 50-nm-thick spherical nanoshells is equivalent to a 1-μm-thick planar nc-Si film. This light-trapping structure could enable the manufacturing of high-throughput ultra-thin film absorbers in a variety of material systems that demand shorter deposition time, less material usage and transferability to flexible substrates.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Electric Conductivity
  • Electric Power Supplies
  • Equipment Design
  • Light
  • Materials Testing
  • Microscopy, Electron, Scanning / methods
  • Nanoshells
  • Nanotechnology / methods*
  • Optics and Photonics
  • Silicon / chemistry*
  • Silicon Dioxide / chemistry
  • Solar Energy
  • Sunlight
  • Temperature

Substances

  • Silicon Dioxide
  • Silicon