Thermally stable rare earth dialkyl complexes supported by a novel bis(phosphinimine)pyrrole ligand

Dalton Trans. 2012 Jul 14;41(26):7873-5. doi: 10.1039/c2dt12485h. Epub 2012 Feb 28.

Abstract

A novel bis(phosphinimine)pyrrole based ligand (HL) and its synthesis are reported. Rare earth dialkyl complexes of the ligand, LLn(CH(2)SiMe(3))(2) (Ln = Er, Lu, Sc), have been prepared and found to exhibit high thermal stability in solution. The protio-ligand and dialkyl lanthanide complexes (Ln = Er, Lu) have been characterised by single crystal X-ray diffraction studies.