Damping factor links periodic focusing and uniform field ion mobility for accurate determination of collision cross sections

Anal Chem. 2012 Mar 20;84(6):2818-24. doi: 10.1021/ac203294q. Epub 2012 Mar 9.

Abstract

The methodology for obtaining accurate ion-neutral collision cross section (Ω) values for peptides and proteins using periodic focusing ion mobility spectrometry (PF IMS) is presented. A mobility dampening factor (represented by the term α) is introduced to account for the relative increase in ion-neutral collisions in PF IMS compared to uniform field ion mobility spectrometry (UF IMS) for equivalent operating conditions. The results show that α may be easily quantified both theoretically and empirically for a specific PF IMS design operating at a given pressure based upon the charge state of the analyte. By simply incorporating an α term into traditional UF IMS expressions, accurate Ω values were obtained with excellent agreement (≤4% difference) compared to UF IMS measurements found in the current literature.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Animals
  • Cattle
  • Horses
  • Ions / chemistry*
  • Mass Spectrometry / methods*
  • Peptides / chemistry*
  • Proteins / chemistry*

Substances

  • Ions
  • Peptides
  • Proteins