Biologically-induced precipitation of sphalerite-wurtzite nanoparticles by sulfate-reducing bacteria: implications for acid mine drainage treatment

Sci Total Environ. 2012 Apr 15:423:176-84. doi: 10.1016/j.scitotenv.2012.02.013. Epub 2012 Mar 11.

Abstract

Several experiments were conducted to evaluate zinc-tolerance of sulfate-reducing bacteria (SRB) obtained from three environmental samples, two inocula from sulfide-mining districts and another inoculum from a wastewater treatment plant. The populations of SRB resisted zinc concentrations of 260 mg/L for 42 days in a sulfate-rich medium. During the experiments, sulfate was reduced to sulfide and concentrations in solution decreased. Zinc concentrations also decreased from 260 mg/L to values below detection limit. Both decreases were consistent with the precipitation of newly-formed sphalerite and wurtzite, two polymorphs of ZnS, forming <2.5-μm-diameter spherical aggregates identified by microscopy and synchrotron-μ-XRD. Sulfate and zinc are present in high concentrations in acid mine drainage (AMD) even after passive treatments based on limestone dissolution. The implementation of a SRB-based zinc removal step in these systems could completely reduce the mobility of all metals, which would improve the quality of stream sediments, water and soils in AMD-affected landscapes.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacteria, Anaerobic / metabolism*
  • Biodegradation, Environmental
  • Chemical Precipitation
  • Environmental Pollutants / chemistry*
  • Industrial Waste*
  • Mining*
  • Nanoparticles / chemistry*
  • Oxidation-Reduction
  • Particle Size
  • Sulfides / chemistry*
  • Waste Management / methods*
  • Zinc / chemistry
  • Zinc Compounds / chemistry*

Substances

  • Environmental Pollutants
  • Industrial Waste
  • Sulfides
  • Zinc Compounds
  • Zinc
  • zinc sulfide