Induction of supramolecular chirality in di-zinc(II) bisporphyrin via tweezer formation: synthesis, structure and rationalization of chirality

Chem Commun (Camb). 2012 Apr 28;48(34):4070-2. doi: 10.1039/c2cc30526g. Epub 2012 Mar 19.

Abstract

Two new supramolecular complexes consisting of an achiral bisporphyrin host and a chiral diamine guest are reported. One shows a remarkably high amplitude bisignate CD signal while the other one shows a very low value. X-ray structure and other spectroscopic investigations of the tweezer complexes clearly rationalize the origin of the optical activity that has so far remained an unresolved issue.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Circular Dichroism
  • Coordination Complexes / chemical synthesis
  • Coordination Complexes / chemistry*
  • Crystallography, X-Ray
  • Diamines / chemical synthesis
  • Diamines / chemistry*
  • Models, Molecular
  • Porphyrins / chemical synthesis
  • Porphyrins / chemistry*
  • Spectrophotometry, Ultraviolet
  • Stereoisomerism
  • Zinc / chemistry*

Substances

  • Coordination Complexes
  • Diamines
  • Porphyrins
  • Zinc